Coherent Ultrafast Polaron Pair Formation In A Conjugated Polymer At Room Temperature

Antonietta De Sio,Ephraim Sommer,Filippo Troiani,Julien Rehault,Margherita Maiuri,Elisa Molinari,Giulio Cerullo,Christoph Lienau

2016 CONFERENCE ON LASERS AND ELECTRO-OPTICS (CLEO)（2016）

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摘要

Ultrafast 2D optical spectroscopy with 10-fs-time-resolution, complemented by density matrix simulations, show that coherent vibronic coupling accelerates polaron-pair formation and results in strongly correlated exciton and polaron-pair dynamics in polythiophene thin films at room temperature.

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关键词

coherent ultrafast polaron pair formation,conjugated polymer,ultrafast 2D optical spectroscopy,time-resolution,density matrix simulations,coherent vibronic coupling,strongly correlated exciton,polaron-pair dynamics,polythiophene thin films,temperature 293 K to 298 K,time 10 fs

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