Imidazolidin-4-ones via (3+2) cycloadditions of aza-oxyallyl cations onto ( E )- N arylideneanilines.

Oznur Eyilcim,Sezin Issever,Nuket Ocal,Scott Gronert,Ihsan Erden

Tetrahedron Letters（2018）

引用 12|浏览4

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摘要

•A new trapping method for aza-oxyallyl cations is described.•Aza-oxyallyl cations undergo novel (3+2) cycloadditions onto N-arylimines.•The products from these reactions are imidazolidin-4-ones.•The reactions are regioselective and in most cases stereoselective.•Experimentally observed regioselectivities are confirmed by DFT calculations.

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关键词

Aza-oxyallyl,Aza-cyclopropanone,N-arylimine,(3+2) cycloaddition,Imidazolidin-4-one

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