Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation.
PHYSICAL REVIEW LETTERS(2016)
Abstract
We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular sigma orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.
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Key words
ultrafast dissociation,molecular orbitals,temporal evolution
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