Bioinspired Total Syntheses of Isospongian-type Diterpenoids (-)-Kravanhins A and C.
CHEMISTRY-AN ASIAN JOURNAL(2016)
摘要
The first bioinspired total syntheses of (-) kravanhins A and C were accomplished from a labdane diterpenoid derivative. The key reactions involve a photooxidation and a one-pot sequential aldol cyclization and lactonization, which provide a new plausible biosynthetic pathway for the kravanhins and other symbiotic members.
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关键词
biosynthesis,natural products,one-pot reactions,terpenoids,total synthesis
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