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Co2+ acireductone dioxygenase: Fe2+ mechanism, Ni2+ mechanism, or something else?

Crystal E. Valdez,Nathan M. Gallup,Anastassia N. Alexandrova

Chemical Physics Letters（2014）

Cited 11|Views8
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Abstract
•Co2+-dependent acireductone dioxygenase exhibits both Fe2+-like and Ni2+-like mechanisms.•Dynamics of reaction may determine the product distribution.•Mixed quantum–classical sampling is required to get the binding of the substrate right.
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Key words
acireductone dioxygenase,co2+,mechanism
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