Coupling of N2O decomposition with CO2 reforming of CH4 in novel cobalt-free BaFe0.9Zr0.05Al0.05O3−δ oxygen transport membrane reactor

Wenyuan Liang,Suresh Kumar Megarajan,Fangyi Liang,Yan Zhang,Guanghu He,Zhenzhen Liu,Heqing Jiang

Chemical Engineering Journal（2016）

引用 28|浏览8

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摘要

•Compared to cobalt-based perovskites, BFZ-Al shows better stability under reducing conditions.•Benefitting from oxygen removal via BFZ-Al membrane, a complete N2O decomposition was achieved.•Simultaneous N2O decomposition and syngas production was achieved in membrane reactor.•BFZ-Al membrane reactor was successfully operated for 100h with fairly stable performance.

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关键词

N2O decomposition,CO2 reforming,Oxygen transport membrane,Cobalt-free perovskite,Membrane reactor

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