Switching on elusive organometallic mechanisms with photoredox catalysis
NATURE(2015)
Abstract
Despite advances in carbon–carbon fragment couplings, the ability to forge carbon–oxygen bonds in a general fashion via nickel catalysis has been largely unsuccessful; here, visible-light-excited photoredox catalysts are shown to provide transient access to Ni( iii ) species that readily participate in reductive elimination, leading to carbon–oxygen coupling.
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Key words
Methodology, Photocatalysis
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