The concerted nature of the cyclization of squalene oxide to the protosterol cation.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION（2013）

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摘要

Concerted A-C ring formation: A concerted, but highly asynchronous, pathway was identified for the formation of rings A-C in the biosynthetic conversion of squalene oxide to the prosterol cation, with ring B being formed in the required boat conformation.

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关键词

carbocations,density functional calculations,reaction mechanisms,squalene,terpenoids

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