Stepwise Coordination Of Pt-Ii-180 Degrees And Pd-Ii-90 Degrees Metal Fragments To The Purine Nucleobase 9-Methylhypoxanthine Affords A Closed Octadecanuclear Pt6pd12 Cluster

Francisca M. Alberti,Witold Zielinski,Marta Morell Cerda,Pablo J. Sanz Miguel,Oliver Troeppner,Ivana Ivanovic-Burmazovic,Bernhard Lippert

CHEMISTRY-A EUROPEAN JOURNAL（2013）

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摘要

Crossing the line: A pH-induced "crossover" in 3D shapes of supramolecular constructs derived from trans(NH3)2Pt(II), [Pd(II)(en)], and the purine model nucleobase 9-methylhypoxanthine (see figure) is reported in which [Pd(en)(H2O)](2+) and [Pd(en)(OH)](+) are the decisive players (en = ethylenediamine).

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关键词

anion binding, host-guest systems, metallacycles, nucleobases

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