AnN-Acyliminium Cyclization Approach to a Total Synthesis of (+)-Cylindricine C
JOURNAL OF ORGANIC CHEMISTRY(2005)
摘要
Details of problems and solutions encountered during the development of an enantioselective total synthesis of (+)-cylindricine C are described here. The total synthesis itself was accomplished in 8 steps, featuring an N-acyliminium. cyclization strategy, the seldom-used Wharton rearrangement, and a key epimerization at C5.
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关键词
total synthesis
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