Mathematical modeling of the kinetics of phenol electrocatalytic hydrogenation over supported Pd–alumina catalyst

Abdelfettah Bannari,Pierre Proulx,Hugues Ménard,Ciprian Mihai Cirtiu

Applied Catalysis A: General（2008）

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摘要

A mathematical model of the electrocatalytic hydrogenation of phenol on a Pd/Al2O3(10%, w/w) catalyst is developed from the chemical kinetic to the fluid mechanical point of view in a laboratory scale cell. The model includes the heterogenous electrochemical steps at the microscopic scale, in a full transient representation of the fluid mechanics in the cell.

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关键词

Kinetic,Adsorption,Langmuir isotherm,Hydrogen adsorption isotherm,Pseudo-second-order model,Catalysis,Electrocatalytic hydrogenation (ECH),Computational fluid dynamics (CFD),Porous media,Multiphase flow

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