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Fluoride Complexation Of Element 104, Rutherfordium

Hiromitsu Haba,Kazuaki Tsukada,Masato Asai,Atsushi Toyoshima,Kazuhiko Akiyama,Ichiro Nishinaka,Masaru Hirata,Tsuyoshi Yaita,Shin-Ichi Ichikawa,Yuichiro Nagame,Ken-Ichiro Yasuda,Yutaka Miyamoto,Tetsuya Kaneko,Shin-Ichi Goto,Sawako Ono,Toshiyuki Hirai,Hisaaki Kudo, Mitsuru Shigekawa,Atsushi Shinohara,Yasuji Oura,Hiromichi Nakahara,Keisuke Sueki,Hidetoshi Kikunaga,Norikazu Kinoshita, Naoya Tsuruga,Akihiko Yokoyama,Minoru Sakama,Shuich Enomoto,Matthias Schädel,Willy Brüchle,Jens V Kratz

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY（2004）

Cited 56|Views53
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Abstract
Fluoride complexation of element 104, rutherfordium (Rf), produced in the (CM)-C-248(O-18,5n)(261)Rf reaction has been studied by anion-exchange chromatography on an atom-at-a-time scale. The anion-exchange chromatographic behavior of Rf was investigated in 1.9-13.9 M hydrofluoric acid together with those of the group-4 elements Zr and Hf produced in the O-18-induced reactions on Ge and Gel targets, respectively. It was found that the adsorption behavior of Rf on anion-exchange resin is quite different from those of Zr and Hf, suggesting the influence of relativistic effects on the fluoride complexation of Rf.
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fluoride,element
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