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Dr. Graessley was a strong proponent of using the fundamental ideas of chain entanglement to understand rheological observations in polymer liquids and crosslinked networks. He designed and conducted many experiments to test hypotheses on what entanglements might be and how they controlled rheology. Nowadays, concepts of entanglement are commonplace and accepted as being broadly useful, however, at the time of his research, in the 1960s and 1970s, it was a highly controversial idea. In his extensive 1974 review, "The Entanglement Concept in Polymer Rheology," (Advances in Polymer Science) he presented early theoretical ideas and experimental evidence for entanglement dynamics in polymeric liquids and in crosslinked networks. Simulations done after his work proved that chain entanglements provide a key contribution to the elastic modulus of polymeric liquids. After moving to emeritus status at Princeton, he completed a two book sequence on Polymeric Liquids & Networks. Volume 1, Structures and Properties, was published in 2004 and Volume 2, Dynamics and Rheology, was published in 2008.
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mag(2006)
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Physics Todayno. 6 (2005)
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