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Research Summary
Our group focuses on bio-inorganic chemistry, specifically on the topic of iron, oxygen and (bio)catalysis. Our research effort, involving a combination of biochemical, synthetic inorganic, and spectroscopic approaches, is aimed at elucidating the oxygen activation mechanisms of nonheme iron enzymes, designing functional models for such enzymes, trapping and characterizing reaction intermediates, and developing bio-inspired oxidation catalysts for green chemistry applications. The pictures illustrate the crystal structure of a recently isolated oxoiron(IV) complex with the oxo atom syn to the methyl groups of the TMC macrocycle and a DFT-calculated structure for a reactive intermediate that we have trapped in our efforts to develop bio-inspired iron catalysts for hydrocarbon oxidation.
Our group focuses on bio-inorganic chemistry, specifically on the topic of iron, oxygen and (bio)catalysis. Our research effort, involving a combination of biochemical, synthetic inorganic, and spectroscopic approaches, is aimed at elucidating the oxygen activation mechanisms of nonheme iron enzymes, designing functional models for such enzymes, trapping and characterizing reaction intermediates, and developing bio-inspired oxidation catalysts for green chemistry applications. The pictures illustrate the crystal structure of a recently isolated oxoiron(IV) complex with the oxo atom syn to the methyl groups of the TMC macrocycle and a DFT-calculated structure for a reactive intermediate that we have trapped in our efforts to develop bio-inspired iron catalysts for hydrocarbon oxidation.
Research Interests
Papers共 766 篇Author StatisticsCo-AuthorSimilar Experts
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Waqas Rasheed, Nabhendu Pal,Ahmed M. Aboelenen,Saikat Banerjee,Williamson N. Oloo,Johannes E. M. N. Klein,Ruixi Fan,Jin Xiong, Yisong Guo,Lawrence Que Jr
JOURNAL OF THE AMERICAN CHEMICAL SOCIETYno. 6 (2024): 3796-3804
Lorna M. Doyle, Roel L.M. Bienenmann,Robert Gericke,Shuangning Xu,Erik R. Farquhar,Lawrence Que,Aidan R. McDonald
Journal of Inorganic Biochemistry (2024): 112583-112583
Proceedings of the National Academy of Sciences of the United States of Americano. 12 (2024): e2319799121-e2319799121
Proceedings of the National Academy of Sciencesno. 12 (2024)
INORGANIC CHEMISTRYno. 4 (2024): 2194-2203
Proceedings of the National Academy of Sciences of the United States of Americano. 51 (2023): e2307950120-e2307950120
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICAno. 51 (2023)
ioChem-BD Computational Chemistry Datasets (2023)
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