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Our research especially targets anions of environmental relevance. We focus on current day challenges including remediation, such as nuclear waste site clean-up, as well as ways to address the looming depletion of the world’s available phosphorus reserves. As a result, we have explored the capture of small oxo anions, halides, and larger carboxylates and polyphosphates. Anions of interest range in shape, from monoatomic to complex polyatomic anions; and charge, from -1 to -12. One goal has been to design anion ligands capable of binding sulfate for nuclear remediation efforts at waste sites such as the National Laboratory at Hanford, in Washington state. While seemingly innocuous, sulfate’s physical properties, e.g., lack of solubility in borosilicate glass and caustic nature, are detrimental to separations efforts. Newer hosts include a urea macrocycle that binds sulfate selectively and a new ion pair host design as shown below.
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Nathalie Busschaert,Clifton J. Stephenson,Kristin Bowman-James,Lyle Isaacs, Benjamin E. Partridge,Ken D. Shimizu,Douglas A. Vander Griend,Kejia Shi, Emmanuel O. Ojah
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