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Buck made enormous contributions to the fields of electroanalytical chemistry and fundamental electrochemistry during his many years as an active researcher. Indeed he is the author/coauthor on more than 240 original research papers, dating back to his earliest work on the first constant-current dual intermediate titrimetric scheme that was published in Analytical Chemistry in1952. In the ‘60s and ‘70s he focused his efforts on the theory of interfacial potential development and selectivity of solid-state and glass membrane electrodes, including very tedious calculations of the potential profiles that exist at electrode/membrane interfaces (using numerical solutions of the Nernst-Planck-Poisson equation). He was one of the very first to apply impedance methods to delineate the charge-transfer kinetics at the interfaces and within the bulk of membrane electrodes, including the development of improved instrumentation to carry out such impedance measurements. As newer organic liquid- and polymer-membrane-based ion-selective electrodes began to emerge in the 1970s, Buck turned his attention to understanding the ion permselectivity of such membranes, including an in-depth effort to define the role of endogenous and exogenous lipophilic counterion sites in preventing interfacial Donnan failure at higher concentrations of analyte ions.He later went on to pioneer the development of novel microfabricated ion and biosensor arrays based on flexible Kapton substrates, and further demonstrated that such devices can be implanted within living heart muscle to provide the first real time measurements of key ions (H+, K+, etc.) and metabolites (e.g., lactate) in such tissue.
Dick Buck’s research contributions go beyond the classical electrochemistry boundaries.Indeed, several of his early academic papers dealt with spark sources for mass spectrometry, spectral deconvolution methods, Raman spectroscopy of adsorbates on electrode surfaces, etc.As one nominating letter writer put it, “these (other) contributions clearly illustrate the great breadth of his knowledge and interests … and the high scholarly quality of his work (electroanalytical and other) over an extended time period makes him especially worthy of receiving SEAC’s highest honor.”
Dick Buck’s research contributions go beyond the classical electrochemistry boundaries.Indeed, several of his early academic papers dealt with spark sources for mass spectrometry, spectral deconvolution methods, Raman spectroscopy of adsorbates on electrode surfaces, etc.As one nominating letter writer put it, “these (other) contributions clearly illustrate the great breadth of his knowledge and interests … and the high scholarly quality of his work (electroanalytical and other) over an extended time period makes him especially worthy of receiving SEAC’s highest honor.”
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IUPAC Standards Online (2016)
Encyclopedia of Surface and Colloid Science, Third Editionpp.3999-4020, (2015)
Electroanalysisno. 3 (2008): 259-269
Robert Gyurcsányi,Ernö Lindner,Géza Nagy, Alessandra Cristalli,Richard Buck,Michael Neuman,Livia Nagy,Stefan Ufer,H Troy Nagle
Biomedical Diagnostic Science (2002)
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